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The road to sustainable use and waste management of plastics in Portugal

《环境科学与工程前沿（英文）》 2022年 第16卷 第1期   页码 5-5 doi: 10.1007/s11783-021-1439-x

摘要：

• Portugal recycles 34% of the 40 kg/hab year of plastic packaging waste.

关键词： Single-use plastics     Plastic packaging     Plastic waste     Waste management     Waste shipment     Lightweight plastic bags    

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Thermal and catalytic pyrolysis of a synthetic mixture representative of packaging plastics residue

Simona Colantonio, Lorenzo Cafiero, Doina De Angelis, Nicolò M. Ippolito, Riccardo Tuffi, Stefano Vecchio Ciprioti

《化学科学与工程前沿（英文）》 2020年 第14卷 第2期   页码 288-303 doi: 10.1007/s11705-019-1875-3

摘要： A synthetic mixture of real waste packaging plastics representative of the residue from a material recovery facility (plasmix) was submitted to thermal and catalytic pyrolysis. Preliminary thermogravimetry experiments coupled with Fourier transform infrared spectroscopy were performed to evaluate the effects of the catalysts on the polymers’ degradation temperatures and to determine the main compounds produced during pyrolysis. The thermal and catalytic experiments were conducted at 370°C, 450°C and 650°C using a bench scale reactor. The oil, gas, and char yields were analyzed and the compositions of the reaction products were compared. The primary aim of this study was to understand the effects of zeolitic hydrogen ultra stable zeolite Y (HUSY) and hydrogen zeolite socony mobil-5 (HZSM5) catalysts with high silica content on the pyrolysis process and the products’ quality. Thermogravimetry showed that HUSY significantly reduces the degradation temperature of all the polymers—particularly the polyolefines. HZSM5 had a significant effect on the degradation of polyethylene due to its smaller pore size. Mass balance showed that oil is always the main product of pyrolysis, regardless of the process conditions. However, all pyrolysis runs performed at 370°C were incomplete. The use of either zeolites resulted in a decrease in the heavy oil fraction and the prevention of wax formation. HUSY has the best performance in terms of the total monoaromatic yield (29 wt-% at 450°C), while HZSM5 promoted the production of gases (41 wt-% at 650°C). Plasmix is a potential input material for pyrolysis that is positively affected by the presence of the two tested zeolites. A more effective separation of polyethylene terephthalate during the selection process could lead to higher quality pyrolysis products.

关键词： packaging plastics waste     plasmix     pyrolysis     zeolite catalyst     degradation temperature    

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ENVIRONMENTAL ATTITUDES AND CONSUMER PREFERENCE FOR ENVIRONMENTALLY-FRIENDLY BEVERAGE PACKAGING: THE

《农业科学与工程前沿（英文）》 2023年 第10卷 第1期   页码 95-108 doi: 10.15302/J-FASE-2022478

摘要：

● Consumer preference for environmentally-friendly beverage packaging was investigated.

关键词： China     consumer preference     food and beverage packaging     green identity label     information treatment     plastics    

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Microbial biodegradation of plastics: Challenges, opportunities, and a critical perspective

《环境科学与工程前沿（英文）》 2022年 第16卷 第12期 doi: 10.1007/s11783-022-1596-6

摘要：

● Health hazards of plastic waste on environment are discussed.

关键词： Plastic-waste     Polymers     Health-hazards     Biodegradation     Microorganisms     Enzymes    

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我国废弃塑料污染防治战略研究

王琪,瞿金平,石碧,陈宁,聂敏,杨双桥

《中国工程科学》 2021年 第23卷 第1期   页码 160-166 doi: 10.15302/J-SSCAE-2021.01.020

摘要：

废弃塑料污染防治是国家战略的重要组成部分。本文全面深入分析我国废弃塑料的来源、回收利用及回收利用技术的现状。在塑料全生命周期评价基础上，提出了我国塑料污染防治全链条解决方案：在技术层面，必须从塑料合成、加工、应用和处理等各环节全方位全链条防治废弃塑料污染，包括塑料制品源头减量，塑料原料及替代产品的开发，塑料制品循环利用的设计，高性能长服役期塑料制品的加工，废弃塑料清洁高效规模化回收利用，终极塑料垃圾的安全处理等；在政府层面，建议加强政府政策引导，落实行政监管；在企业层面，建立有效回收机制，明确生产者、经营者、消费者的回收责任，为废弃塑料污染防治提供政策及技术建议；在公众层面，提高公民环保意识，全民参与治理。采用上述提出的我国塑料污染防治全链条解决方案，可以促进我国塑料工业和国民经济绿色可持续发展。

关键词： 废弃塑料     环境污染     防治措施     回收利用     全链条治理    

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Multi-Component Resource Recycling from Waste Light-Emitting Diode Under Hydrothermal Condition: Plastic

Yongliang Zhang,Lu Zhan,Zhenming Xu,

《工程（英文）》 doi: 10.1016/j.eng.2023.04.008

摘要： Light emitting diodes (LEDs) have accounted for most of the lighting market as the technology matures and costs continue to reduce. As a new type of e-waste, LED is a double-edged sword, as it contains not only precious and rare metals but also organic packaging materials. In previous studies, LED recycling focused on recovering precious and strategic metals while ignoring harmful substances such as organic packaging materials. Unlike crushing and other traditional methods, hydrothermal treatment can provide an environment-friendly process for decomposing packaging materials. This work developed a closed reaction vessel, where the degradation rate of plastic polyphthalamide (PPA) was close to 100%, with nano-TiO2 encapsulated in plastic PPA being efficiently recovered, while metals contained in LED were also recycled efficiently. Besides, the role of water in plastic PPA degradation that has been overlooked in current studies was explored and speculated in detail in this work. Environmental impact assessment revealed that the proposed recycling route for waste LED could significantly reduce the overall environmental impact compared to the currently published processes. Especially the developed method could reduce more than half the impact of global warming. Furthermore, this research provides a theoretical basis and a promising method for recycling other plastic-packaged e-waste devices, such as integrated circuits.

关键词： Waste LED     Hydrothermal treatment     Recycling     Plastic PPA degradation     Packaging materials    

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Pyrolysis of WEEE plastics using catalysts produced from fly ash of coal gasification

Marika Benedetti, Lorenzo Cafiero, Doina De Angelis, Alessandro Dell’Era, Mauro Pasquali, Stefano Stendardo, Riccardo Tuffi, Stefano Vecchio Ciprioti

《环境科学与工程前沿（英文）》 2017年 第11卷 第5期 doi: 10.1007/s11783-017-0998-3

摘要： Catalytic pyrolysis of thermoplastics extracted from waste electrical and electronic equipment (WEEE) was investigated using various fly ash-derived catalysts. The catalysts were prepared from fly ash by a simple method that basically includes a mechanical treatment followed by an acid or a basic activation. The synthesized catalysts were characterized using various analytical techniques. The results showed that not treated fly ash (FA) is characterized by good crystallinity, which in turn is lowered by mechanical and chemical treatment (fly ash after mechanical and acid activation, FAMA) and suppressed almost entirely down to let fly ash become completely amorphous (fly ash after mechanical and basic activation FAMB). Simultaneously, the surface area resulted increased. Subsequently, FA, FAMB and FAMA were used in the pyrolysis of a WEEE plastic sample at 400°C and their performance were compared with thermal pyrolysis at the same temperature. The catalysts principally improve the light oil yield: from 59wt.% with thermal pyrolysis to 83 wt.% using FAMB. The formation of styrene in the oil is also increased: from 243 mg/g with thermal pyrolysis to 453 mg/g using FAMB. As a result, FAMB proved to be the best catalyst, thus producing also the lowest and the highest amount of char and gas, respectively.

关键词： Waste electrical and electronic equipment (WEEE) plastic mixture     Pyrolysis     Catalyst     Fly ash     Oil    

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Anthocyanins/chitosan films doped by nano zinc oxide for active and intelligent packaging: comparison

《化学科学与工程前沿（英文）》 2023年 第17卷 第6期   页码 704-715 doi: 10.1007/s11705-022-2270-z

摘要： The multifunctional films was prepared by blending chitosan and nano-ZnO with purple tomato anthocyanins or black wolfberry anthocyanins. The properties of films functioned by anthocyanins source and nano-ZnO content were studied. It was found purple tomato anthocyanins showed more significant color change against pH than black wolfberry anthocyanins. The nano-ZnO were widely dispersed in matrix and enhanced the compatibility of anthocyanins with chitosan. However, the anthocyanins source influenced the properties of the films more slightly than nano-ZnO addition. The tensile strength, antioxidant and antibacterial effects of the chitosan films dramatically increased after cooperated by nano-ZnO and anthocyanins, which also enhanced with increase of nano-ZnO content, whereas the elongation at break of the composite films decreased. Especially, the anthocyanin and nano-ZnO promoted the antibacterial activity of films synergistically. Composite films made from black wolfberry anthocyanins exhibited higher mechanical performance than those made from purple tomato anthocyanins but weaker antibacterial effects. The purple tomato anthocyanins/chitosan and nano-ZnO/purple tomato anthocyanins/chitosan films effectively reflected pork spoilage, changing their colors from dark green to brown, indicating the potential for applications in active and intelligent food packaging.

关键词： bio-based     multifunction     colorimetric indicator     active and intelligent packaging    

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Improvement potential of today’s WEEE recycling performance: The case of LCD TVs in Belgium

Paul Vanegas, Jef R. Peeters, Dirk Cattrysse, Wim Dewulf, Joost R. Duflou

《环境科学与工程前沿（英文）》 2017年 第11卷 第5期 doi: 10.1007/s11783-017-1000-0

摘要： Waste of electrical and electronic equipment (WEEE) constitutes one of the most relevant waste streams because of the quantity and presence of valuable materials. However, there is limited knowledge on the resource potential of urban mining WEEE, as data on material composition, and the efficiency of current recycling treatments are still scarce. In this article, an evaluation of the recycling performance at a national level for one of the fastest growing e-waste streams: LCD TVs is carried out through the following four steps. Firstly, material characterisation is performed by means of sampling of the waste stream. Secondly, a material flow analysis is conducted by evaluating the separation performance of a recycling plant in Belgium. Thirdly, the recovered economic value and avoided environmental impact (EI) of the analysed recycling system is assessed. Finally, the potential of urban mining for Belgium is forecasted. The analysis shows that while recycling performance for ferrous metals and aluminium are relatively high; there is substantial room to better close the material loops for precious metals (PM) and plastics. PMs and plastics account for 66 % of the economic value in LCD TVs and 57% of the EI. With the current, commonly applied recycling technology only one-third of the PM and housing plastics are recycled; meaning that for these materials, at a national level for Belgium, there is a potential for improvement that represents 3.3 million euros in 2016 and 6.8 million euros in 2025.

关键词： Recycling     Waste of electrical and electronic equipment (WEEE)     Material flow analysis     LCD TVs     Precious metals     Plastics    

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Prediction of cutting forces in machining of unidirectional glass fiber reinforced plastics composite

Surinder Kumar GILL, Meenu GUPTA, P. S. SATSANGI

《机械工程前沿（英文）》 2013年 第8卷 第2期   页码 187-200 doi: 10.1007/s11465-013-0262-x

摘要：

Machining of plastic materials has become increasingly important in any engineering industry subsequently the prediction of cutting forces. Forces quality has greater influence on components, which are coming in contact with each other. So it becomes necessary to measure and study machined forces and its behavior. In this research work, experimental investigations are conducted to determine the effects of cutting conditions and tool geometry on the cutting forces in the turning of the unidirectional glass fiber reinforced plastics (UD-GFRP) composites. In this experimental study, carbide tool (K10) having different tool nose radius and tool rake angle is used. Experiments are conducted based on the established Taguchi’s technique L18 orthogonal array on a lathe machine. It is found that the depth of cut is the cutting parameter, which has greater influence on cutting forces. The effect of the tool nose radius and tool rake angles on the cutting forces are also considerably significant. Based on statistical analysis, multiple regression model for cutting forces is derived with satisfactory coefficient (R2). This model proved to be highly preferment for predicting cutting forces.

关键词： unidirectional glass fiber reinforced plastics (UD-GFRP) composites     machining     cutting forces (tangential     feed and radial force)     ANOVA     regression modeling     carbide tool (K10)    

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Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1570-3

摘要：

● Collaborative treatment of plastics and OS was established to improve oil quality.

关键词： Oily sludge     Pyrolysis     Polyethylene     H/Ceff ratio     Oil quality    

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塑料加工成型技术的最新研究进展

瞿金平

《中国工程科学》 2011年 第13卷 第10期   页码 58-68

摘要：

依据塑料工业发展低耗、高效、环保型“绿色”加工成型技术的重大需求，随着塑料塑化输运方法的不断演变与创新，在塑料动态加工成型方法和设备的基础上提出和研究了基于拉伸流变的塑料加工成型方法和技术，着重讨论了拉伸形变支配的叶片挤压系统中塑料塑化输运过程、叶片挤压系统的技术特征和叶片塑化输运技术的应用。研究结果表明，与传统技术及设备相比较，这种新技术及设备具有加工历程缩短50 %以上、加工能耗降低30 %左右、混合混炼效果好、制品质量提高、对物料适应性广等优异的技术性能。同时发现，新技术及设备在多相多组份复合材料、剪切热敏感高分子材料等物料体系的加工方面具有独特优势。

关键词： 塑料     加工成型     拉伸形变     塑化输运    

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用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

《中国工程科学》 2002年 第4卷 第6期   页码 56-62

摘要：

对静电键合、体硅直接键合和界面层辅助键合等三种体硅键合技术，整片操作、局部操作和选择保护等三种密封技术，以及这些技术用于微电子机械系统的密封作了评述，强调在器件研究开始时应考虑封装问题，具体技术则应在保证器件功能和尽量减少芯片复杂性两者之间权衡决定。

关键词： 体硅键合技术     薄膜密封技术     微电子机械系统封装技术    

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基于玻璃通孔的Ka波段宽带滤波封装天线 Research Article

方针1,2,张继华1,2,3,高莉彬1,2,陈宏伟1,2,李文磊1,2,梁天鹏1,2,蔡旭东1,2,蔡星周3,贾惟聪3,郭欢3,李勇3

《信息与电子工程前沿（英文）》 2023年 第24卷 第6期   页码 916-926 doi: 10.1631/FITEE.2200573

摘要： 以玻璃封装材料和玻璃通孔技术为基础，提出一种新的Ka波段(33 GHz)滤波封装天线(FPA)，该天线具有宽频带和高滤波响应特点。与传统封装材料(印刷电路板、低温共烧陶瓷、硅等)相比，玻璃通孔更适合小型化技术(毫米波三维封装器件)，具有优越的微波性能。玻璃基板通过键合技术可实现三维高密度互联，其热膨胀系数与硅相当。此外，玻璃基板的堆叠实现了高密度互连，并与微电子技术兼容。该天线辐射贴片由贴片天线和反射系数几乎互补的带通滤波器(BPF)组成。BPF单元有3对λg/4槽(缺陷微带结构)和两对λg/2 U形缝隙(缺陷地结构)。该天线实现了大带宽和高辐射效率，这可能与玻璃基板的叠加和玻璃通孔馈电有关。此外，引入4个辐射零值可有效提高阻带内的抑制水平。为验证所提设计性能，对33 GHz宽带滤波天线进行优化、调试和测量。天线的工作带宽为29.4‒36.4 GHz (|S11|<−10 dB)，阻抗匹配带宽高达21.2%，阻带抑制水平大于16.5 dB。该天线实际增益为~6.5 dBi，辐射效率为~89%。

关键词： 滤波封装天线；玻璃通孔；三维封装器件；激光键合    

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预应力FRP加固工程结构技术研究进展

卢亦焱,陈娟,黄银燊,吴涛

《中国工程科学》 2008年 第10卷 第8期   页码 40-44

摘要：

围绕国内外预应力FRP加固技术的研究现状以及最新进展，从预应力FRP加固混凝土结构、预应力FRP加固钢结构、预应力FRP加固中关键技术的研究等方面进行了综述。试验研究表明：预应力FRP加固混凝土能显著提高构件的开裂荷载、屈服荷载和极限荷载，改善受弯构件在长期荷载的力学性能，提高构件的疲劳寿命；预应力CFRP加固钢梁后，其屈服荷载和极限荷载相对于对比梁都有明显的提高，其提高的程度随着预应力CFRP的用量和预应力水平的提高而增大；预应力CFRP加固对钢梁的刚度提高作用也比较明显，对低强度的钢材，提高效果更明显；采用预应力FRP加固工程结构的关键问题在于预应力的施加体系、预应力控制值、预应力损失和端部的锚固。

关键词： 纤维增强塑料     加固技术     混凝土结构     钢结构     研究进展    

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标题 作者 时间 类型 操作

The road to sustainable use and waste management of plastics in Portugal

期刊论文

Thermal and catalytic pyrolysis of a synthetic mixture representative of packaging plastics residue

Simona Colantonio, Lorenzo Cafiero, Doina De Angelis, Nicolò M. Ippolito, Riccardo Tuffi, Stefano Vecchio Ciprioti

期刊论文

ENVIRONMENTAL ATTITUDES AND CONSUMER PREFERENCE FOR ENVIRONMENTALLY-FRIENDLY BEVERAGE PACKAGING: THE

期刊论文

Microbial biodegradation of plastics: Challenges, opportunities, and a critical perspective

期刊论文

我国废弃塑料污染防治战略研究

王琪,瞿金平,石碧,陈宁,聂敏,杨双桥

期刊论文

Multi-Component Resource Recycling from Waste Light-Emitting Diode Under Hydrothermal Condition: Plastic

Yongliang Zhang,Lu Zhan,Zhenming Xu,

期刊论文

Pyrolysis of WEEE plastics using catalysts produced from fly ash of coal gasification

Marika Benedetti, Lorenzo Cafiero, Doina De Angelis, Alessandro Dell’Era, Mauro Pasquali, Stefano Stendardo, Riccardo Tuffi, Stefano Vecchio Ciprioti

期刊论文

Anthocyanins/chitosan films doped by nano zinc oxide for active and intelligent packaging: comparison

期刊论文

Improvement potential of today’s WEEE recycling performance: The case of LCD TVs in Belgium

Paul Vanegas, Jef R. Peeters, Dirk Cattrysse, Wim Dewulf, Joost R. Duflou

期刊论文

Prediction of cutting forces in machining of unidirectional glass fiber reinforced plastics composite

Surinder Kumar GILL, Meenu GUPTA, P. S. SATSANGI

期刊论文

Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis

期刊论文

塑料加工成型技术的最新研究进展

瞿金平

期刊论文

用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

期刊论文

基于玻璃通孔的Ka波段宽带滤波封装天线

方针1,2,张继华1,2,3,高莉彬1,2,陈宏伟1,2,李文磊1,2,梁天鹏1,2,蔡旭东1,2,蔡星周3,贾惟聪3,郭欢3,李勇3

期刊论文

预应力FRP加固工程结构技术研究进展

卢亦焱,陈娟,黄银燊,吴涛

期刊论文